Magnetic fluctuations caused by the nuclear spins of a host crystal are often the leading source of decoherence for many types of solid-state spin qubit. In group-IV materials, the spin-bearing nuclei are sufficiently rare that it is possible to identify and control individual host nuclear spins. This work presents the first experimental detection and manipulation of a single 29 Si nuclear spin. The quantum non-demolition (QND) single-shot readout of the spin is demonstrated, and a Hahn echo measurement reveals a coherence time of T2 = 6.3(7) ms -in excellent agreement with bulk experiments. Atomistic modeling combined with extracted experimental parameters provides possible lattice sites for the 29 Si atom under investigation. These results demonstrate that single 29 Si nuclear spins could serve as a valuable resource in a silicon spin-based quantum computer.The presence of non-zero nuclear spins in a host crystal lattice is known to induce decoherence in a central spin qubit through mechanisms such as spectral diffusion [1]. This "nuclear bath" is the primary source of decoherence for 31 P electron and nuclear spin qubits in silicon [2,3], nitrogen-vacancy (NV) centers in diamond [4], as well as for GaAs-based quantum dot spin qubits [5,6]. However, for semiconductors composed of majority spin-zero isotopes (such as silicon and carbon), the low abundance of spin-carrying nuclei allows to resolve the hyperfine couplings of individual nuclei with a central electronic spin, permitting the detection and manipulation of single nuclear spins. This has led to the demonstration of a quantum register for the spin of a NV center in diamond, where the electronic spin state can be stored in individual nuclei [7] and read out in single shot [8]. Quantum error correction protocols have been implemented within these nuclear spin registers [9,10], showing their potential to implement surface-code based quantum computing architectures [11]. Natural silicon contains a 4.7% abundance of the spin-carrying (I = 1/2) 29 Si isotope which, in combination with a localized electron spin, could in principle be used as quantum register or ancilla qubit equivalently to 13 C in NV-diamond. In addition, the 29 Si nuclear spin has itself been championed as a quantum bit in an "allsilicon" quantum computer [12,13].Here we present the first experimental demonstration of single-shot readout, coherent control, and measurement of the coherence properties of an individual 29 Si nuclear spin in natural Si. All measurements were performed with a magnetic field B 0 = 1.77 T, in a dilution refrigerator with electron temperature T el ≈ 250 mK. This work follows from previous experiments where the electron [2] and nuclear [3] spins of a single 31 P donor were detected using a compact nanoscale device [14] consisting of ion-implanted phosphorus donors [15], tunnel-coupled to a silicon MOS single- electron transistor (SET) [16]. Spin control was achieved through microwave and RF excitations generated by an arXiv:1408.1347v1 [cond-mat.mes-hall]