“…Consequently, MBE growth studies of Bi2Se3 and Bi2Te3 thin films have been carried out on a variety of substrates, e.g., Si(001) and (111), [13] GaN(001), [14] GaAs(001) and (111), [12,15] CdTe(111), [16] SiC(001), [17] as well as on lattice-matched InP(111) [18] and, more recently, Bi2Se3 was grown on Ge(111). [19,20] From a technological point of view, the integration of TIs with long-spindiffusion-length semiconductor materials such as germanium seems to be a very promising solution for the current CMOS (complementary metal-oxide-semiconductor) technology limitations. [21] One of the challenges for monolithic device integration of TIs is their weak bonding to most substrates, originating from the van der Waals (vdW)-type interaction between film and substrate.…”