Temporal variations of volume and mass in the magma chambers of Sakurajima Volcano were modeled using leveling and relative gravity data collected around the volcano during the eruptive period from 1975 to 1992, to reveal a physical mechanism for the excessive gravity increase observed at the volcano. The following two deflation sources were estimated from the leveling data: a deeper source of -4.2 ×106 m3/yr located 8000 m deep beneath Aira Caldera, and a shallower source of -7.25 × 105 m3/yr located 3600 m deep beneath the center of Sakurajima Volcano. These deflation sources cannot fully explain the gravity increase of up to 15.75 microGal/yr observed at the volcano, because a gravity increase of only <3.27 microGal/yr is expected from the two deflation sources. After the effect of the deflation sources was subtracted from the observed gravity change, the residual gravity of up to 12.48 microGal/yr was then modeled by a point mass increase under the volcano. The estimated rate of the mass increase was 4.50 × 1010 kg/yr, and the position of the point mass agreed with that of the shallower magma chamber within its error range. This result suggests that the shallower magma chamber gained mass despite the chamber deflation during the 1975-1992 eruptive period, and can be quantitatively explained by the accumulation of degassed magma in the shallower chamber. Our modeling results also suggest the importance of gravimetry in addition to crustal deformation observations in quantifying the rate of magma mass supply, because the magma supply to the deeper chamber was calculated to be +5.39 × 1010 kg/yr from the gravity and leveling data, which is six times greater than that calculated from the leveling data only.