SrCr x Fe 12Àx O 19 (x = 0.0, 0.1, 0.3, 0.5, 0.7, 0.9) hexaferrites were prepared by a microwave-hydrothermal method and subsequently sintered at 950°C for 90 min using the microwave sintering method. The results show that, with increasing Cr 3+ content, the lattice parameters changed anisotropically. The average grain sizes of sintered samples were in the range of 280 nm to 660 nm. The saturation magnetization systematically decreased with increasing Cr 3+ doping, but the coercivity values increased. The electrical resistivity (log q) decreased linearly with increasing temperature up to a certain temperature known as the transition temperature (T c ), and T c decreased with further increase (x > 0.5) of the Cr 3+ content. This decrease in log q and the activation energy (E g ) is due to electron hopping and occupancy of doped ions at different lattice sites. We found that the dielectric constant and dielectric loss for all the samples decreased with the Cr 3+ content. The structural, magnetic, and electrical properties of Cr 3+ -doped SrFe 12 O 19 hexaferrites have thus been investigated.