2002
DOI: 10.1364/josab.19.000102
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High-intensity third-harmonic generation

Abstract: The azimuthal dependence of third-order and cascaded second-order nonlinear coupling are used to measure the relative contributions of each to direct third-harmonic generation in ␤-barium borate. This enabled the measurement of the values of 10(3) , 11 (3) , and 16(3) relative to the known ij (2) . Finally, conversion efficiencies to 3 of up to 6% from a single crystal were achieved with a femtosecond chirped-pulse-amplification laser with 200 GW/cm 2 in collimated beams.

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Cited by 74 publications
(63 citation statements)
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“…Radiation of the second harmonic, generated as a result of 'asynchronous' (not phase-matched) process involving the second-order nonlinearity, interacts with the pump radiation, leading to sum-frequency generation of the third harmonic. The results for the THG effect in the  -BaB 2 O 4 crystal cut at the phase matching angle for the case of direct generation with the third-order nonlinearity have been reported by different scientific groups [2,3]. They differ in the magnitudes of the cascaded and direct contributions to the THG.…”
Section: Introductionmentioning
confidence: 90%
See 1 more Smart Citation
“…Radiation of the second harmonic, generated as a result of 'asynchronous' (not phase-matched) process involving the second-order nonlinearity, interacts with the pump radiation, leading to sum-frequency generation of the third harmonic. The results for the THG effect in the  -BaB 2 O 4 crystal cut at the phase matching angle for the case of direct generation with the third-order nonlinearity have been reported by different scientific groups [2,3]. They differ in the magnitudes of the cascaded and direct contributions to the THG.…”
Section: Introductionmentioning
confidence: 90%
“…As shown in [2], a considerable contribution to the process of phase-matched thirdharmonic generation (THG) using nonlinearity of the third order in uniaxial crystals is originates from the cascaded THG. Radiation of the second harmonic, generated as a result of 'asynchronous' (not phase-matched) process involving the second-order nonlinearity, interacts with the pump radiation, leading to sum-frequency generation of the third harmonic.…”
Section: Introductionmentioning
confidence: 99%
“…However, a relative contribution of the two processes could be different. In some cases, the direct THG process is stronger (see, e.g., Feve, Boulanger, and Guillien [2000]), in other cases the cascading THG process is dominant (see, e.g., Banks, Feit, and Perry [2002]; Bosshard, Gubler, Kaatz, Mazerant, and Meier [2000]). …”
Section: Third-harmonic Multistep Processesmentioning
confidence: 99%
“…One of the ways to separate the contribution of the two nonlinearities and express of χ (3) eff,dir in terms of the product (d eff,I )(d eff,II ) is to use the azimuthal (Banks, Feit, and Perry [2002]) or input polarization (Kim and Yoon [2002]) dependence of χ (3) eff,dir and χ (3) eff,casc . The other way is to compare the TH signal obtained under the condition ∆k THG −→ 0 with the TH signal obtained under one of the conditions ∆k SHG −→ 0 or ∆k SFG −→ 0, where the signal is only proportional to the factor |χ (3) eff,casc | 2 (Akhmanov, Meisner, Parinov, Saltiel, and Tunkin [1977]; Chemla, Begley, and Byer [1974]), and calculate χ (3) eff,dir ; however this procedure gives two possible values due to an indeterminate sign.…”
Section: Measurement Of the χ (3) -Tensor Componentsmentioning
confidence: 99%
“…To that end, we generated 262 nm pulses through third harmonic generation using two type-I beta-barium borate (BBO) crystals, as described in detail by Zohrabi 18 and others. 19,20 This 262 nm laser beam is directed toward the detector through a diverging lens and a flat mirror such that it illuminates the whole detector, as shown in Fig. 1(a).…”
mentioning
confidence: 99%