Amorphous
indium–gallium–zinc oxide (a-IGZO)
has become a standard channel ingredient of switching/driving
transistors in active-matrix organic light-emitting diode (AMOLED)
televisions. However, mobile AMOLED displays with a high pixel density
(≥500 pixels per inch) and good form factor do not often employ a-IGZO transistors due to their modest mobility (10–20
cm2/(V s)). Hybrid low-temperature polycrystalline silicon
and oxide transistor (LTPO) technology is being adapted in high-end
mobile AMOLED devices due to its ultralow power consumption and excellent
current drivability. The critical issues of LTPO (including a complicated
structure and high fabrication costs) require a search for alternative
all-oxide thin-film transistors (TFTs) with low-cost processability
and simple device architecture. The atomic layer deposition (ALD)
method is a promising route for high-performance all-oxide TFTs due
to its unique features, such as in situ cation composition tailoring
ability, precise nanoscale thickness controllability, and excellent
step coverage. Here, we report an in-depth comparative investigation
of TFTs with indium–gallium oxide (IGO)/gallium–zinc
oxide (GZO) and indium–zinc oxide (IZO)/GZO heterojunction
stacks using an ALD method. IGO and IZO layers with different compositions
were tested as a confinement layer (CL), whereas the GZO layer was
used as a barrier layer (BL). Optimal IGO/GZO and IZO/GZO channels
were carefully designed on the basis of their energy band properties,
where the formation of a quasi-two-dimensional electron gas (q2DEG)
near the CL/BL interface is realized by rational design of the band
gaps and work-functions of the IGO, IZO, and GZO thin films. To verify
the effect of q2DEG formation, the device performances and stabilities
of TFTs with CL/BL oxide heterojunction stacks were examined and compared
to those of TFTs with a single CL layer. The optimized device with
the In0.75Zn0.25O/Ga0.80Zn0.20O stack showed remarkable electrical performance: μFE of 76.7 ± 0.51 cm2/(V s), V
TH of −0.37 ± 0.19 V, SS of 0.13
± 0.01 V/dec, and I
ON/OFF of 2.5
× 1010 with low operation voltage range of ≥2
V and excellent stabilities (ΔV
TH of +0.35, −0.67, and +0.08 V for PBTS, NBIS, and CCS, respectively).
This study suggests the feasibility of using high-performance ALD-derived
oxide TFTs (which can compete with the performance of LTPO transistors)
for high-end mobile AMOLED displays.