“…In recent years, mid-infrared (MIR) lasers in the region of 2.7-3 μm have attracted much attention because of their wide applications in the fields of atmospheric monitoring, medical surgery, remote sensing, and scientific research [1][2][3][4][5]. At present, the 2.7-3 μm rare-earth laser crystals have been widely investigated, and various laser crystals with excellent performances have realized laser output in this spectral region, such as Er:YAG (2.94 μm) [6], Er,Pr:GYSGG (2.79 μm) [7,8], Cr,Yb,Ho:YSGG (2.842 μm, 2.888 μm, 2.926 μm, 2.962 μm, 2.973 μm, 3.057 μm) [9], and Ho:YAP (2.844 μm, 2.855 μm, 2.856 μm, 2.920 μm, 3.017 μm) [10] crystals, et al Although the 2.7-3 μm wavelength range is a vibrational absorption band of water, there also exist fine spectral wavebands which have only very weak water absorption, especially at the wavelength of 2.911 μm.…”