2022
DOI: 10.1039/d2tc03148e
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Highly stable and controllable lasing actions from PVDF encapsulated CsPbBr3 perovskite microcrystals

Abstract: Halide perovskite (HP)-based optoelectronics, particularly lasers, have attracted considerable attention thanks to their outstanding low threshold, and tunable bandgaps. Surface coating is one of the most common strategies for significantly...

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Cited by 5 publications
(3 citation statements)
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“…As shown in Table , introducing long-chain and zwitterionic ligands to passivate the surface of QDs has acquired research focus to improve the stability of QDs for their application in electrical injection devices. However, the ligand is highly dynamically bound to the surface of the QDs and has limited resistance to external environments (such as light and heat) . Compared with molecular-state ligands, polymer/inorganic coatings have higher stability to regulate the dynamic binding. However, most polymers have a low thermal stability, , and with a core–shell structure, it is necessary to consider whether the lattices of the core and shell match . In addition, the use of polymers or inorganic shells to coat QDs is complicated and costly, which is not conducive to large-scale synthesis.…”
Section: Introductionmentioning
confidence: 99%
“…As shown in Table , introducing long-chain and zwitterionic ligands to passivate the surface of QDs has acquired research focus to improve the stability of QDs for their application in electrical injection devices. However, the ligand is highly dynamically bound to the surface of the QDs and has limited resistance to external environments (such as light and heat) . Compared with molecular-state ligands, polymer/inorganic coatings have higher stability to regulate the dynamic binding. However, most polymers have a low thermal stability, , and with a core–shell structure, it is necessary to consider whether the lattices of the core and shell match . In addition, the use of polymers or inorganic shells to coat QDs is complicated and costly, which is not conducive to large-scale synthesis.…”
Section: Introductionmentioning
confidence: 99%
“…By means of time-resolved terahertz spectroscopy CsPbBr 3 NCs have been found to possess excellent free carrier performance, with carrier mobilities of up to 4500 cm 2 V −1 s −1 and diffusion lengths greater than 9.2 µm, making for ideal intrinsic transport properties [14]. Thus, halide perovskite holds great value for optoelectronic applications and offers a wide scope 2 of 13 of prospects in high-efficiency solar cells [16][17][18], sensitive photodetectors [19][20][21], lowthreshold lasers [22][23][24], light-emitting diodes (LEDs) [25][26][27], scintillators [28][29][30], and bioimaging systems [31][32][33]. Among the multitude of applications, metal halide perovskite is particularly impressive in the field of solar cells.…”
Section: Introductionmentioning
confidence: 99%
“…By means of time-resolved terahertz spectroscopy, CsPbBr3 NCs were discovered to boast extremely high free carrier dynamics, with carrier mobilities of up to 4500 cm 2 V -1 s -1 and diffusion lengths greater than 9.2 μm, which render their intrinsic transport properties ideal [14]. Thus, halide perovskite holds great value for optoelectronic applications and offers a wide scope of prospects in high-efficiency solar cells [16][17][18], sensitive photodetectors [19][20][21], low-threshold lasers [22][23][24],light-emitting diodes (LEDs) [25][26][27], scintillators [28][29][30], and bioimaging systems [31][32][33]. Among the multitude of applications, metal halide perovskite is particularly impressive in the field of solar cells.…”
Section: Introductionmentioning
confidence: 99%