2016
DOI: 10.1103/physreva.94.050501
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Hydrogen molecular ions for improved determination of fundamental constants

Abstract: The possible use of high-resolution rovibrational spectroscopy of the hydrogen molecular ions H + 2 and HD+ for an independent determination of several fundamental constants is analyzed. While these molecules had been proposed for metrology of nuclear-to-electron mass ratios, we show that they are also sensitive to the radii of the proton and deuteron and to the Rydberg constant at the level of the current discrepancies colloquially known as the proton size puzzle. The required level of accuracy, in the 10 −12… Show more

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Cited by 60 publications
(57 citation statements)
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“…Using counter-propagating laser beams with a narrow linewidth, the Lamb Dicke regime may be reached in the present apparatus, such that first-order Doppler broadening is entirely eliminated, while all other systematic effects could be controlled below the 1 × 10 −13 uncertainty level. Such spectroscopy would allow more stringent tests of molecular theory and QED, tighter bounds on new physics at the Ångström scale, a competitive determination of the proton-electron mass ratio and even contribute to the determination of several other fundamental constants including the Rydberg constant, the deuteron-electron mass ratio, and the proton and deuteron charge radii [41].…”
Section: Conclusion Implications and Outlookmentioning
confidence: 99%
See 1 more Smart Citation
“…Using counter-propagating laser beams with a narrow linewidth, the Lamb Dicke regime may be reached in the present apparatus, such that first-order Doppler broadening is entirely eliminated, while all other systematic effects could be controlled below the 1 × 10 −13 uncertainty level. Such spectroscopy would allow more stringent tests of molecular theory and QED, tighter bounds on new physics at the Ångström scale, a competitive determination of the proton-electron mass ratio and even contribute to the determination of several other fundamental constants including the Rydberg constant, the deuteron-electron mass ratio, and the proton and deuteron charge radii [41].…”
Section: Conclusion Implications and Outlookmentioning
confidence: 99%
“…For example, in Refs. [22,41] an experiment was proposed in which the (v, L) = (0, 3) → (9, 3) line in HD + is addressed through a two-photon transition with nearly degenerate photons. Using counter-propagating laser beams with a narrow linewidth, the Lamb Dicke regime may be reached in the present apparatus, such that first-order Doppler broadening is entirely eliminated, while all other systematic effects could be controlled below the 1 × 10 −13 uncertainty level.…”
Section: Conclusion Implications and Outlookmentioning
confidence: 99%
“…As was pointed out already some time ago [3], and recently discussed more extensively [4], if the theory would be sufficiently precise, the spectroscopy of HMI may be used for determining of the fundamental physical constants such as the protonto-electron mass ratio. The ionization energy of HMI is also of high importance for the determination of ionization and dissociation energies of the hydrogen molecule from spectroscopic studies [5][6][7] as well as for the determination of atomic masses of light nuclei [8][9][10].On the experimental side there are many new projects started, which are now oriented towards Doppler-free spectroscopy with accuracy targeted to 1 ppt (one part per trillion) or better [4,[11][12][13]. These perspectives bring strong motivation for theory.…”
mentioning
confidence: 99%
“…From the theoretical point of view the HMI is one of the simplest nonintegrable quantum system, which still allows very accurate numerical treatment. As was pointed out already some time ago [3], and recently discussed more extensively [4], if the theory would be sufficiently precise, the spectroscopy of HMI may be used for determining of the fundamental physical constants such as the protonto-electron mass ratio. The ionization energy of HMI is also of high importance for the determination of ionization and dissociation energies of the hydrogen molecule from spectroscopic studies [5][6][7] as well as for the determination of atomic masses of light nuclei [8][9][10].…”
mentioning
confidence: 99%
“…These are currently at lower precision than other methods but prospects exist that competitive values can be derived from molecular spectroscopy. Similarly Karr et al [14] recently discussed the possibility of determining R ∞ using H + 2 (or HD + ) transitions as an alternative to atomic hydrogen spectroscopy. Even for the neutral system of molecular hydrogen, the determination of r p from spectroscopy is projected to be achievable, from the ongoing efforts in both calculation [15] and experiments [16].…”
mentioning
confidence: 99%