Artificial spin ice systems have opened experimental windows into a range of model magnetic systems through the control of interactions among nanomagnet moments. This control has previously been enabled by altering the nanomagnet size and the geometry of their placement. Here we demonstrate that the interactions in artificial spin ice can be further controlled by including a soft ferromagnetic underlayer below the moments. Such a substrate also breaks the symmetry in the array when magnetized, introducing a directional component to the correlations. Using spatially resolved magneto-optical Kerr effect microscopy to image the demagnetized ground states, we show that the correlation of the demagnetized states depends on the direction of underlayer magnetization. Further, the relative interaction strength of nearest and next-nearest neighbors varies significantly with the array geometry. We exploit this feature to induce frustration in an inherently unfrustrated square lattice geometry, demonstrating new possibilities for effective geometries in two dimensional nanomagnetic systems.
Custom-designed artificial magnetic materials provide model platforms for studying a variety of fundamental problems in magnetism and also form the basis for applications such as non-volatile memory and spin-based logic. Examples include magnetic multilayers and heterostructures wherein interlayer and interfacial exchange coupling yields new magnetic behavior relevant to spintronic applications [1], continuous ferromagnetic films interfaced with patterned ferromagnetic arrays that allow systematic control over pinning of magnetic domain walls [2], and nanoscale ferromagnetic elements with mixed anisotropy that allow the engineering of spin frustration and spin texture [3]. Artificial spin ice (ASI) is another interesting example of a custom-designed magnetic material, in which interacting arrays of lithographically-defined single domain nanomagnets are arranged in frustrated two-dimensional geometries (e.g. triangular and kagome) [4, 5]. A variety of fundamental phenomena have been studied in ASIs, including the physics of Dirac strings and magnetic monopoles [6-10], the interplay between frustration and thermal fluctuations [11, 12], and geometric [13, 14], and topological [15] and vertex [16] frustration. ASI systems are also candidates for reconfigurable magnonics and neuromorphic computing. Perpendicular ansitropy ASIs, in which the individual islands have perpendicular magnetic anisotropy (PMA) with moments pointing normal to the plane of the structure, [17, 18] DE-SC0020162.