We report an order-of-magnitude reduction in the electric field required for domain nucleation in 1 mol % MgO-doped near-stoichiometric and 5 mol % MgO-doped congruently grown lithium niobate crystals induced by illumination from a focused continuous wave laser beam at wavelengths of 514, 488, and 457 nm. A smaller decrease of 31% is also observed for undoped congruently grown crystals. The effect is independent of the visible wavelengths explored. Periodically poled lithium niobate ͑PPLN͒ has been successfully exploited for various quasi-phase-matched nonlinear applications.1 The efficiency of the quasi-phase-matching is limited, however, by the susceptibility of congruently grown lithium niobate to photorefractive damage 2,3 induced during room temperature operation with high power and short-pulsed lasers, restricting the applicability of congruently grown lithium niobate. This limitation can be significantly reduced by the use of magnesium-doped ͑MgO-doped͒ lithium niobate which exhibits a higher resistance to such photorefractive effects, 4,5 a lower coercive field for ferroelectric domain reversal, 6 and comparable nonlinear optical coefficients 7 for use in frequency conversion processes.
8Electric field poling with structured electrodes is a routinely employed technique for fabrication of PPLN, but the period lengths obtainable with this technique are currently limited to a few micrometers. However, many applications require smaller structures, hence alternative methods for domain patterning are currently under investigation in our laboratory. Light-induced domain patterning may be a suitable technique to overcome this size limitation. Previous lightassisted poling experiments which take advantage of an ultraviolet-light-induced change in the coercive field to transfer a patterned light distribution into an equivalent domain structure in bulk crystals have already been reported for undoped and MgO-doped lithium niobate 9-11 crystals. The use of focused visible laser light, which has the effect of reducing the coercive field through a light-induced space charge field, has recently been demonstrated to directly write domain structures of ϳ2 m dimensions in undoped lithium niobate crystals.
12Here we investigate the influence of the illumination by visible light from an Ar-ion laser on the electric field required to induce domain nucleation ͑nucleation field͒ in MgO-doped and undoped lithium niobate crystals. Domain nucleation is defined here as the first observation of 180°i nverted domain seeds that subsequently extend through the crystal on further application of an electric field. It is worth noting that the nucleation field is less than the coercive field, which is often defined by a poling current exceeding some arbitrary threshold, as in Ref. 11.Several types of commercially available z-cut single crystal lithium niobate samples from different crystal suppliers were investigated. The two types of congruently grown crystals used were 300-m-thick undoped ͑YamPure͒ and 500-m-thick 5 mol % MgO-doped ͑YamM...