Higher depths at the millimeter scale (1-2 mm), along with greater magnitudes, have been reported after the NLSP of Ti6Al4V titanium alloy, [2,10] 2024, [11] 6061, [12] and 7075 [13] aluminum alloys. Elaborated laser systems with large power densities are currently required to increase the peak pressure to enable a high input of energy (slightly over 10 GW cm -2 ) during the interaction between the incident laser and metals. [14] The critical power density threshold for the confinement layer breakdown is validated to limit the possible peak pressure. [15][16][17] Changing the wavelength of the incident laser from 1064 to 532 nm decreases the breakdown threshold of the confining water layers from 10 to 6 GW cm -2 , and the maximum peak pressure from ≈5.5 to 4.5 GPa. [18,19] Compressive residual stresses can also be generated deep below the peened surface by multiple or overlapping laser pulses. [20,21] The reduced attenuation of the shock wave indicates an increased depth for the plastic-deformed layer during subsequent peening, while the affected depths usually reach saturated border values within three to five impacts. [22,23] Additionally, femtosecond laser shock peening is applied to induce a shallower affected depth and a limited compressive layer owing to the high instantaneous power density. [24] It is necessary to increase the surface optical absorption and associated energy conversion at higher affected depths in NLSP. The surface optical absorption property determines the thermal energy fraction, [25,26] with a value of ≈0.2 utilized in investigations. [27,28] In this case, optical absorption is defined by the surface morphology of the metal rather than its intrinsic absorptance. [29] Various absorption mechanisms with different optical behaviors are found in the structures induced using lithographic and chemical techniques. [30,31] These essentially originate from selective absorption responses such as the surface plasmon resonance, magnetic-polariton, geometric optical response, and metamaterial resonances. [29,[32][33][34] A nanoscale structure and laser-induced periodic surface structure can enhance the absorption of laser energy by the reconstruction of surface electromagnetic distributions. [35] The absorption of light is enhanced on structured surfaces by multiple reflections based on the angular dependence of Fresnel absorption. [35] The absorption spectrum of femtosecond laser treated surfaces increased sharply over a wide range of wavelengths of incident Laser shock peening is conducted to enhance the mechanical properties of metals. Efficient optical absorption of metal surface is desirable to increase the laser shock peening depth. In this work, a method is proposed to regulate the absorption behavior by surface colorizing to increase the affected depth and magnitude of nanosecond laser shock peening (NLSP). Colorized samples are fabricated with high absorption of 400-1500 nm, which is 89% higher than that of un-colorized samples. This regulated optical response is attributed to the multi-ref...