Ferromagnetic ͑FM͒ resonance and magnetization curve measurements were performed at room temperature for a polycrystalline Ni 81 Fe 19 coupled to NiO. It was observed that the shape of the angular variation of the resonance field is frequency dependent, with the curve at 9.65 GHz typical for a strongly exchange-coupled bilayer, while the 34.0 GHz curve is characteristic for relatively weak interactions. Numerical simulations of the resonance field and of the hysteresis loop shift, carried out through the domain wall formation model, as well as the resonance linewidth data indicated that there must be two fractions in the antiferromagnetic part of the interface, with stable and unstable grains. Only the stable grains contribute to the exchange bias. In our sample, whether an interfacial antiferromagnetic grain is stable or not is predominantly determined by the strength of the exhange coupling between this grain and the adjacent FM domain. The stable antiferromagnetic grains, whose contribution is sensed by the resonance experiment, are the smaller ones, which are more strongly coupled to the ferromagnet than the larger grains. The exchange-bias phenomenon, 1 which results from the interfacial coupling between ferromagnetic ͑FM͒ and antiferromagnetic ͑AF͒ materials, has been extensively studied in the last decade, motivated by fundamental and practical interests. One of the reasons for the continued interest is the fact that different experimental techniques may yield different exchange anisotropy values. [2][3][4][5][6][7][8][9] In some cases, this was assigned to the fact that the measurements are performed on different sets of samples. 4 Another source for the discrepancy could be the reliability of the model used in the experimental data interpretation. 8 It has also been shown 9 that the exchange-bias field values derived from magnetization and ferromagnetic resonance ͑FMR͒ measurements, must, in general, give different values in the framework of the domain-wall formation ͑DWF͒ model which assumes formation of a planar domain wall at the AF side of the interface with the reversal of the FM orientation. 8,10 Recent FMR studies on exchange-coupled NiFe films showed the importance of the magnetic state of the AF part of the interface. McMichael et al.11 used FMR to study the relaxation behavior of polycrystalline AF layer and found that the stability of the AF order is critical to the existence of the exchange bias. Relaxation related to thermally driven reversal of the AF grains in such systems has also been observed.
12,13The aim of the present work was to apply the phenomenological approach for the DWF model recently developed by our group 9 on a real exchange coupled system. The paper describes FMR and magnetization measurements of a bilayer of Permalloy ͑Py͒ ͑here, Ni 81 Fe 19 ) exchange-coupled to NiO. The striking frequency dependence of the FMR angular variation has been related to the relaxation behavior of the interfacial AF grains.The sample under investigation was deposited by rf magnetron sputterin...