Completing this work has certainly been a journey. Along the way there were triumphs and setbacks, tremendous gains and devastating losses. Many things are quite different now than they were over six years ago when I first found myself a fresh grad student in old Tate hall. The research presented here has all taken place against a backdrop of changing personal, political, and societal conditions. I have only managed to navigate this all due to aid of many people, and I owe each of them my thanks for the influence they have had in my life. Because you are so numerous and I so forgetful, I am certain to neglect some of you, but here goes... First I thank Prisca Cushman and Vuk Mandic who have together steered the course of the SuperCDMS group at UMN. Their scientific, professional, and personal guidance have helped shape me into a better physicist. In particular I thank my advisor Vuk for his calm and insightful manner and superb mentorship. Your steady hand has been a great help and comfort to me at many times, certainly more than I have let show. Thanks also to the post-docs I had the pleasure of working with at UMN, including Hassan Chagani, Matt Fritts, and Anthony Villano. Hassan and Matt, you helped me learn how to operate a dilution fridge with enough confidence to only occasionally wake bolt upright in the middle of the night in fear that I had left some important valve open and lost all the mix! From what I understand now, that is actually a sign of a reasonable level of competence, so thank you! Matt and Anthony, you helped me to learn many of the nuts and bolts of the particular blend of astrophysical, solid state, and experimental particle physics that is DM research. You have also shown through your diligent work and attention to detail how essential, but also how hard it is to produce good, solid, and valuable scientific results. While I am a better researcher for having worked with each of you, more importantly, I value you both as friends.