“…During the past few years, extensive studies have been conducted on Nd:CNGG, including continuous-wave (CW) laser oper-ation on the three main transitions from 4 F 3/2 to 4 I 13/2 , 4 I 11/2 , and 4 I 9/2 [2][3][4][5][6]; generation of visible radiation through intracavity frequency doubling or sum-frequency mixing [7][8][9][10]; and mode-locked laser action [11]. Besides Nd:CNGG, ytterbium doped CNGG (Yb:CNGG) has also been developed in 2007 [12], and has proven to be a promising laser medium for both CW and pulsed (Qswitched or mode-locked) laser applications [13][14][15][16]. Very recently, a new different kind of Nd doped disordered garnet crystal, Nd:GYSGG, was also developed, showing promising potential in generating CW, Q-switched, and mode-locked laser operation [17,18].…”