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Several researchers observed a significant increase in water flow through graphene-based nanocapillaries. As graphene sheets are flexible (Wang and Shi 2015 Energy Environ. Sci. 8 790–823), we represent nanocapillaries with a deformable channel-wall model by using the small displacement structural-mechanics and perturbation theory presented by Gervais et al (2006 Lab Chip 6 500–7), and Christov et al (2018 J. Fluid Mech. 841 267–86), respectively. We assume the lubrication assumption in the shallow nanochannels, and using the microstructure of confined water along with slip at the capillary boundaries and disjoining pressure (Neek-Amal et al 2018 Appl. Phys. Lett. 113 083101), we derive the model for deformable nanochannels. Our derived model also facilitates the flow dynamics of Newtonian fluids under different conditions as its limiting cases, which have been previously reported in literature (Neek-Amal et al 2018 Appl. Phys. Lett. 113 083101; Gervais et al 2006 Lab Chip 6 500–7; Christov et al 2018 J. Fluid Mech. 841 267–86 ; White 1990 Fluid Mechanics; Keith Batchelor 1967 An Introduction to Fluid Dynamics ; Kirby 2010 Micro-and Nanoscale Fluid Mechanics: Transport in Microfluidic Devices). We compare the experimental observations by Radha et al (2016 Nature 538 222–5) and MD simulation results by Neek-Amal et al (2018 Appl. Phys. Lett. 113 083101) with our deformable-wall model. We find that for channel-height H o < 4 Å, the flow-rate prediction by the deformable-wall model is 5%–7% more compared to Neek-Amal et al (2018 Appl. Phys. Lett. 113 083101) well-fitted rigid-wall model. These predictions are within the errorbar of the experimental data as shown by Radha et al (2016 Nature 538 222–5), which indicates that the derived deformable-wall model could be more accurate to model Radha et al (2016 Nature 538 222–5) experiments as compared to the rigid-wall model. Using the model, we study the effect of the flexibility of graphene sheets on the flow rate. As the flexibility α increases (or corresponding thickness T and elastic modulus E of the wall decreases), the flow rate also increases. We find that the flow rate scales as m ˙ flexible ∼ α 0 for ( α Δ p W / E H o ) ≪ 1 ; m ˙ flexible ∼ α for ( α Δ p W / E H o ) ∼ O ( 10 − 1 ) ; and m ˙ flexible ∼ α 3 for ( α Δ p W / E H o ) ∼ O ( 1 ) , respectively. We also find that, for a given thickness T , the percentage change in flow rate in the smaller height of the channel is more than the larger height of the channels. As the channel height decreases for the given reservoir pressure and thickness, the Δ m ˙ / m ˙ increases with H o − 1 followed by H o − 3 after a height-threshold. Further, we investigate how the applied pulsating pressure influences the flow rate. We find that due to the oscillatory pressure field, there is no change in the averaged mass flow rate in the rigid-wall channel, whereas the flow rate increases in the flexible channels with the increasing magnitude of the oscillatory pressure field. Also, in flexible channels, depending on the magnitude of the pressure field, either of the steady or oscillatory or both kinds of pressure field, the averaged mass flow rate dependence varies from Δ p to Δ p 4 as the pressure field increases. The flow rate in the rigid-wall channel scales as m ˙ rigid ∼ Δ p , whereas for the deformable-wall channel it scale as m ˙ flexible ∼ Δ p for ( α Δ p W / E H o ) ≊ 0 , m ˙ flexible ∼ Δ p 2 for ( α Δ p W / E H o ) ∼ O ( 10 − 1 ) , and m ˙ flexible ∼ Δ p 4 for ( α Δ p W / E H o ) ∼ O ( 1 ) . We find that both the flexibility of the graphene sheet and the pulsating pressure fields to these flexible channels intensify the rapid flow rate through nano/Angstrom-size graphene capillaries.
Several researchers observed a significant increase in water flow through graphene-based nanocapillaries. As graphene sheets are flexible (Wang and Shi 2015 Energy Environ. Sci. 8 790–823), we represent nanocapillaries with a deformable channel-wall model by using the small displacement structural-mechanics and perturbation theory presented by Gervais et al (2006 Lab Chip 6 500–7), and Christov et al (2018 J. Fluid Mech. 841 267–86), respectively. We assume the lubrication assumption in the shallow nanochannels, and using the microstructure of confined water along with slip at the capillary boundaries and disjoining pressure (Neek-Amal et al 2018 Appl. Phys. Lett. 113 083101), we derive the model for deformable nanochannels. Our derived model also facilitates the flow dynamics of Newtonian fluids under different conditions as its limiting cases, which have been previously reported in literature (Neek-Amal et al 2018 Appl. Phys. Lett. 113 083101; Gervais et al 2006 Lab Chip 6 500–7; Christov et al 2018 J. Fluid Mech. 841 267–86 ; White 1990 Fluid Mechanics; Keith Batchelor 1967 An Introduction to Fluid Dynamics ; Kirby 2010 Micro-and Nanoscale Fluid Mechanics: Transport in Microfluidic Devices). We compare the experimental observations by Radha et al (2016 Nature 538 222–5) and MD simulation results by Neek-Amal et al (2018 Appl. Phys. Lett. 113 083101) with our deformable-wall model. We find that for channel-height H o < 4 Å, the flow-rate prediction by the deformable-wall model is 5%–7% more compared to Neek-Amal et al (2018 Appl. Phys. Lett. 113 083101) well-fitted rigid-wall model. These predictions are within the errorbar of the experimental data as shown by Radha et al (2016 Nature 538 222–5), which indicates that the derived deformable-wall model could be more accurate to model Radha et al (2016 Nature 538 222–5) experiments as compared to the rigid-wall model. Using the model, we study the effect of the flexibility of graphene sheets on the flow rate. As the flexibility α increases (or corresponding thickness T and elastic modulus E of the wall decreases), the flow rate also increases. We find that the flow rate scales as m ˙ flexible ∼ α 0 for ( α Δ p W / E H o ) ≪ 1 ; m ˙ flexible ∼ α for ( α Δ p W / E H o ) ∼ O ( 10 − 1 ) ; and m ˙ flexible ∼ α 3 for ( α Δ p W / E H o ) ∼ O ( 1 ) , respectively. We also find that, for a given thickness T , the percentage change in flow rate in the smaller height of the channel is more than the larger height of the channels. As the channel height decreases for the given reservoir pressure and thickness, the Δ m ˙ / m ˙ increases with H o − 1 followed by H o − 3 after a height-threshold. Further, we investigate how the applied pulsating pressure influences the flow rate. We find that due to the oscillatory pressure field, there is no change in the averaged mass flow rate in the rigid-wall channel, whereas the flow rate increases in the flexible channels with the increasing magnitude of the oscillatory pressure field. Also, in flexible channels, depending on the magnitude of the pressure field, either of the steady or oscillatory or both kinds of pressure field, the averaged mass flow rate dependence varies from Δ p to Δ p 4 as the pressure field increases. The flow rate in the rigid-wall channel scales as m ˙ rigid ∼ Δ p , whereas for the deformable-wall channel it scale as m ˙ flexible ∼ Δ p for ( α Δ p W / E H o ) ≊ 0 , m ˙ flexible ∼ Δ p 2 for ( α Δ p W / E H o ) ∼ O ( 10 − 1 ) , and m ˙ flexible ∼ Δ p 4 for ( α Δ p W / E H o ) ∼ O ( 1 ) . We find that both the flexibility of the graphene sheet and the pulsating pressure fields to these flexible channels intensify the rapid flow rate through nano/Angstrom-size graphene capillaries.
A clear visualization of the physical processes of spatially confined ns laser induced atmospheric air plasma within a rectangular glass cavity using optical imaging is presented. The occurrence of various processes starting from the early plasma and shock wave expansion dynamics to shock reflection at the cavity boundaries and compression of the plasma due to reflected shockwaves is studied using defocused shadowgraphy and self-emission imaging techniques. Experimentally, we evidenced that the counter propagating reflected primary shockwaves (PSW) interact with the expanding plasma generating a secondary shockwave (SSW) which compresses the plasma core, modifying the plasma morphology resulting in enhanced plasma parameters. The numerical simulations performed via the two-dimensional hydrodynamic (2D-HD) FLASH codes, revealed that the number density increases up to a maximum of 3.6 times compared to the unconfined plasma. The input laser pulse energy and the aspect ratio of the cavity is observed to play a dominant role in the confinement and compression of the plasma.
Several researchers observed a significant increase in water flow through graphene-based nanocapillaries [1-2]. As graphene sheets are flexible [3], we represent nanocapillaries with a deformable channel-wall model by using the small displacement structural-mechanics and perturbation theory presented by Gervais et al.[4], and Christov et al.[5], respectively. We assume the lubrication assumption in the shallow nanochannels, and using the microstructure of confined water along with slip at the capillary boundaries and disjoining pressure [2], we derive the model for deformable nanochannels. Our derived model also facilitates the flow dynamics of Newtonian fluids under different conditions as its limiting cases, which have been previously reported in literature [2,4-8]. We compare the experimental observations by Radha et al.[1] and MD-simulation results by Neek-Amal et al.[2] with our deformable-wall model. We find that for channel-height $H_o < 4$~\AA, the flow-rate prediction by the deformable-wall model is 5-7~\% more compared to [2] well-fitted rigid-wall model. These predictions are within the errorbar as shown by [1], which indicates that the derived deformable-wall model could be more accurate to model [1] experiments as compared to the rigid-wall model. Using the model, we study the effect of flexibility of graphene sheets on the flow rate. As the flexibility $\alpha$ increases (corresponding thickness $\mathcal{T}$ and elastic modulus $E$ of the wall decreases), the flow rate also increases. We find that the flow rate scales as $\dot{m}_{\text{flexible}}\sim \alpha^0 $ for $\Big (\alpha \Delta pW/EH_o \Big ) \ll 1$; $\dot{m}_{\text{flexible}}\sim \alpha $ for $\Big (\alpha \Delta pW/EH_o \Big ) \sim O(10^{-1})$; and $\dot{m}_{\text{flexible}}\sim \alpha^3 $ for $\Big (\alpha \Delta pW/EH_o \Big ) \sim O(1)$, respectively. We also find that, for a given thickness $\mathcal{T}$, the percentage change in flow rate in the smaller height of the channel is more than the larger height of the channels. As the channel height decreases for the given reservoir pressure and thickness, the $\Delta \dot{m}/\dot{m}$ increases with $H_o^{-1}$ followed by $H_o^{-3}$ after a height-threshold. Further, we investigate how the applied pulsating pressure influences the flow rate. We find that due to the oscillatory pressure field, there is no change in the averaged mass flow rate in the rigid-wall channel, whereas the flow rate increases in the flexible channels with the increasing magnitude of the oscillatory pressure field. Also, in flexible channels, depending on the magnitude of the pressure field, either of the steady or oscillatory or both kinds of pressure field, the averaged mass flow rate dependence varies from $\Delta p$ to $\Delta p^4$ as the pressure field increases. The flow rate in the rigid-wall channel scales as $\dot{m}_{\text{rigid}}\sim \Delta p $, whereas for the deformable-wall channel it scale as $\dot{m}_{\text{flexible}}\sim \Delta p $ for $ (\alpha \Delta pW/EH_o ) \approxeq 0$, $\dot{m}_{\text{flexible}}\sim \Delta p^2 $ for $ (\alpha \Delta pW/EH_o ) \sim O(10^{-1})$, and $\dot{m}_{\text{flexible}}\sim \Delta p^4 $ for $ (\alpha \Delta pW/EH_o ) \sim O(1)$. We find that both the flexibility of the graphene sheet and the pulsating pressure fields to these flexible channels intensify the rapid flow rate through nano/Angstrom-size graphene capillaries.
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