Abstract. Fine particulate matter (PM2.5) has altered the radiation balance on Earth
and raised environmental and health risks for decades but has only been
monitored widely since 2013 in China. Historical long-term PM2.5
records with high temporal resolution are essential but lacking for both
research and environmental management. Here, we reconstruct a site-based
PM2.5 dataset at 6 h intervals from 1960 to 2020 that combines
long-term visibility, conventional meteorological observations, emissions,
and elevation. The PM2.5 concentration at each site is
estimated based on an advanced machine learning model, LightGBM, that takes
advantage of spatial features from 20 surrounding meteorological stations.
Our model's performance is comparable to or even better than those of
previous studies in by-year cross validation (CV) (R2=0.7) and
spatial CV (R2=0.76) and is more advantageous in long-term records
and high temporal resolution. This model also reconstructs a 0.25∘ × 0.25∘, 6-hourly, gridded PM2.5 dataset by
incorporating spatial features. The results show PM2.5 pollution
worsens gradually or maintains before 2010 from an interdecadal scale but
mitigates in the following decade. Although the turning points vary in
different regions, PM2.5 mass concentrations in key regions decreased
significantly after 2013 due to clean air actions. In particular, the annual
average value of PM2.5 in 2020 is nearly the lowest since 1960. These
two PM2.5 datasets (publicly available at
https://doi.org/10.5281/zenodo.6372847, Zhong et al., 2022) provide spatiotemporal variations at
high resolution, which lay the foundation for research studies associated
with air pollution, climate change, and atmospheric chemical reanalysis.