“…In response to the rapid development of electric vehicles and portable electronic devices, accelerating the charging/discharging rates of lithium-ion batteries has become one of the most critical issues, in addition to increasing energy density. − For instance, the required time to fully charge the car batteries, typically 1–3 h, should hopefully be shortened to be compared with that for filling up petrol motor cars in several minutes. Applying high voltages to the conventional batteries shortens the charging period to several tens of minutes, although consequently causing the unfavorable energy (voltage) loss, self-heating, and degradation of battery components. , Former studies revealed that optimizing the crystal structures of the electrode-active materials, controlling the nanoscale geometry, and addition of nanocarbons such as graphene were effective to achieve the outstanding charge/discharge rates over 10–100 C ( x C corresponds to a rate to fully charge/discharge a cell in 1/ x hours). − Still, most of the newly developed materials are yet to be commercialized because of the strict criteria for practical use, such as cyclability, energy density, voltage, reliability, toxicity, and mass producibility.…”