“…Subsequently, resonance lidars have been used for active, altitude-resolved soundings (Bowman et al, 1969), and most recently, satellite-borne spectrometers, detecting scattered sunlight or nightglow, have provided a near global coverage (e.g., Gumbel et al, 2007). So far, the alkali metals, sodium, lithium, and potassium (e.g., Eska et al, 1998;Jegou et al, 1980;Qian & Gardner, 1995); the alkaline earth metals, calcium (e.g., Gerding et al, 2000;Granier et al, 1985) and magnesium (e.g., Correira et al, 2008;Langowski et al, 2015); and the transition metal, iron (e.g., Alpers et al, 1993;Bills & Gardner, 1990;Chu et al, 2011), have been investigated. The metal ions Ca + and Mg + have also been observed by ground-based lidar (e.g., Gerding et al, 2000) and from space (Langowski et al, 2015), respectively.…”