In Tokyo, the annual average suspended particulate matter (SPM) and PM 2.5 concentrations have decreased in the past two decades. The present study quantitatively evaluated these decreasing trends using data from air-pollution monitoring stations. Annual SPM and PM 2.5 levels at 83 monitoring stations and hourly SPM and PM 2.5 levels at four monitoring stations in Tokyo, operated by the Tokyo Metropolitan Government, were used for analysis, together with levels of co-pollutants and meteorological conditions. Traffic volume in Tokyo was calculated from the total traveling distance of vehicles as reported by the Ministry of Land, Infrastructure, Transport, and Tourism. High positive correlations between SPM levels and nitrogen oxide levels, sulfur dioxide levels, and traffic volume were determined. The annual average SPM concentration declined by 62.6% from 59. Significant positive correlations were found between traffic volumes and SPM or PM 2.5 , but the average concentrations of SPM and PM 2.5 concentration per traffic volume have also decreased over the decade studied. These results suggest that reductions in traffic volumes as well as improvements in engine design and the installation of exhaust gas treatment systems may have improved air quality.