“…Two-dimensional (2D) crystalline nanomaterials have generated widely growing interest for diverse applications on mechanically soft flexible substrates owing to their generally inert surface, high elasticity, and thickness scalability down to a monolayer, which represents the ideal limit for electrostatic control, optical transparency, and bendability. − Over the past decade, graphene has been the foremost 2D atomic crystal investigated for flexible nanoelectronics with substantial advances in large-scale synthesis, device mobility, cutoff frequency, strain tolerance, and mechanical robustness. − ,− However, its lack of a bandgap results in a transistor that cannot be switched off by a gate voltage, an indispensable requirement for the vast majority of circuits in modern electronic systems . Recently, transitional metal dichalcogenides (TMDs) such as MoS 2 and WSe 2 have emerged as suitable layered semiconductors that offer a sizable bandgap attractive for low-power electronics. ,,,, Nonetheless, despite promising theoretical prospects, , experimental TMD device mobilities have been relatively low, less than 50 cm 2 /V·s on flexible substrates so far, ,− a value comparable to established amorphous materials such as metal oxide semiconductors that have transitioned into application products. − …”