“…Historically, several approaches have been explored to increase their performance such as, participation ratio engineering [3]-typically resulting in bigger qubits-as well as optimal control [4,5], shielding [6] and signal filtering [7]. In contrast, the number of advancements based on understanding microscopic origin of decoherence and energy loss-including the judicious increase of the materials toolbox-is rather limited [8,9], with most published work focusing on only a few well documented materials such as Al [10][11][12][13][14][15], Nb [16][17][18][19][20], TiN [21,22], NbN [23,24], NbTiN [25][26][27], granular-Al [28,29], Re [30] and In [31]. Only recently, the suite of materials for superconducting quantum technology was further expanded, markedly resulting in qubit relaxation times as high as 0.5 ms for 2D transmon qubits by using α-tantalum (α-Ta) [32,33].…”