One of environmental crises facing the world is due to rubber auto tires destruction pollution. Tires' exploitation in vehicles consumes 6 % of the world's energy and causes 5 % of carbon dioxide emissions; it releases up to 10 % of the microplastic pollution found in oceans.We designed a new rubber nanocomposite self-assembled from hard and soft elastomer matrixes: the polybutadiene with two hydroxy chain ends reacted with 4,4'-diphenylmethane diisocyanate to form segmented polyurethane. This system first undergoes a self-assembly, forming well-defined nanoscale hard domains distributed in the soft matrix. Then, cross-linking between the soft segments was accomplished by a controlled radiation method, resulting in the double network elastomer (DN-E). Remarkably, DN-E exhibited the lowest reported loss factor value at 60 o C. The index of energy dissipation in the rolling tire This article is protected by copyright. All rights reserved. 3 demonstrated a prominent reduction of 72 %, accomplished with 88 % decrease in energy loss, and 85 % less wear loss, as compared with best earlier reported commercial tires. These new double-network materials open a new prospective for design and fabrication of ultralow energy-consumption and strong abrasion-resistance elastomers, which establishes a milestone for the development of the next generation of green low pollution tires causing much less energy dissipation.