“…Gas concentrations (CH 4 , CO 2 , C 2 H 6 , H 2 S) were measured in real time using laser spectrometers (Picarro Inc., Santa Clara, CA, USA), (2) computational signal processing and geochemical analysis were used to distinguish oil and gas emissions from biogenic, naturally occurring sources, or other anthropogenic emissions, (3) we conducted a back-trajectory analysis to attribute emission anomalies observed on-road to specific upwind sites, (4) volumetric emissions rates were estimated via a point-source Gaussian Dispersion Model (GDM). Each of these steps, and uncertainties therein, have been explained previously 9 , 17 , 18 . Thus, only a brief overview is included in the next three subsections.…”