1994
DOI: 10.1016/s0167-2991(08)63921-x
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Methylation of Organic Model Compounds by Methane over Substituted Aluminophosphate Molecular Sieves

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Cited by 4 publications
(3 citation statements)
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“…As mentioned earlier in the introduction section, previous studies by Long et al [2,13] have demonstrated using 13 C labelled methane that the source of methyl groups in the methylated aromatic products of the reaction of methane with naphthalene, toluene and phenol in a high pressure batch reactor over substituted aluminophosphate molecular sieves was predominantly the methane reactant. This then implied actual activation of the methane molecule.…”
Section: Discussionmentioning
confidence: 85%
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“…As mentioned earlier in the introduction section, previous studies by Long et al [2,13] have demonstrated using 13 C labelled methane that the source of methyl groups in the methylated aromatic products of the reaction of methane with naphthalene, toluene and phenol in a high pressure batch reactor over substituted aluminophosphate molecular sieves was predominantly the methane reactant. This then implied actual activation of the methane molecule.…”
Section: Discussionmentioning
confidence: 85%
“…These substrates would be those that have previously been reported to undergo direct methylation with methane over aluminophosphate catalysts such as naphthalene, toluene and phenol [2,13]. Other substrates that model petroleum, coal and liquefaction residue structures (eg benzene, diphenylmethane, biphenyl, diphenyl sulfide, diphenyl ether and dinaphthol) [3] that have also been demonstrated to have methane incorporated into them over Cu-beta, H-beta and CuZSM-5 should also be investigated.…”
Section: Concluding Remarks and Suggestions For Future Workmentioning
confidence: 99%
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