The laser deflector is a crucial device used to change the direction of light beam propagation in various fields, including lithography, lidar, and scanning. In this paper, we conduct a systematic study of two KTa (1−x) Nb x O 3 (KTN) crystals that use different physical deflection mechanisms. We analyze their dielectric properties, entropy, domain structure, and deflection performance. We also address the drawback of the small deflection angle of the compositional gradient KTN deflector crystal by proposing a new temperature-compensated temperature control strategy to improve its deflection performance. The gradient temperature control mechanism maximizes the dielectric constant in different regions of the KTN crystals, leading to a threefold (10.67 mrad) increase in deflection angle compared to conventional uniform temperature control equipment. This optimized temperature control mechanism can significantly enhance the practical application of KTN crystals, providing a new avenue for achieving a large deflection angle beam deflector.