2006
DOI: 10.1039/b514912f
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Molecular conductors with the common and robust building block (BEDT-TTF)2NP (NP = [FeNO(CN)5]2–) but different band filling

Abstract: Two new organic conductors based on BEDT-TTF radical cation salts with the [FeNO(CN) 5 ] 22 anion have been synthesized. b0-(BEDT-TTF) 2 [FeNO(CN) 5 ] (1) and b0-(BEDT-TTF) 3 [FeNO(CN) 5 ]?EG (2) have been characterized by single-crystal X-ray diffraction, electrical resistance measurements, and electronic band-structure calculations. A detailed comparison of 1 and 2 with b0-(BEDT-TTF) 4 A[FeNO(CN) 5 ] 2 (3) is reported. 2 and 3 are organic metals stable down to low temperatures while 1 is a semiconductor. Ana… Show more

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