Morphology and structure of diamond-like carbon film induced by picosecond laser ablation

Takabayashi, Keisuke; Takahashi, Takashi; Tsuchiya, Eibon; Mimura, Kazuki; Yamamoto, Yoshiyuki; Kobayashi, Yohei; Tomita, Takuro; Yamaguchi, Makoto

doi:10.1007/s00339-022-05980-5

Appl. Phys. A

2022

DOI: 10.1007/s00339-022-05980-5

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Morphology and structure of diamond-like carbon film induced by picosecond laser ablation

Keisuke Takabayashi

Takashi Takahashi²,

Eibon Tsuchiya³

et al.

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2024

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A multi-method study of femtosecond laser modification and ablation of amorphous hydrogenated carbon coatings

Hirahara,

Bonse,

Krüger

et al. 2024

Appl. Phys. A

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We present a study on femtosecond laser treatment of amorphous hydrogen-containing carbon coatings (a-C:H). The coatings were deposited on silicon wafers by a plasma-assisted chemical vapour deposition (PA-CVD), resulting in two different types of material with distinct properties (referred to as “absorbing” and “semi-transparent” coatings in the following). The samples were laser-treated with single fs-laser pulses (800 nm center wavelength, 35 fs pulse duration) in the ablative regime. Through a multi-method approach using topometry, Raman spectroscopy, and spectroscopic imaging ellipsometry, we can identify zones and thresholds of different fluence dependent effects and have access to the local dielectric function. The two coating materials react significantly different upon laser treatment. We determined the (non-ablative) modification threshold fluence for the absorbing coating as $$3.6\times {10}^{-2}$$ 3.6 × 10 - 2 Jcm−2 and its ablation threshold as 0.22 Jcm−2. The semi-transparent coating does not show such a low-fluence modification but exhibits a characteristic interference-based intra-film ablation mechanism with two distinguishable ablation thresholds at 0.25 and 0.28 Jcm−2, respectively. The combination of tailored layer materials and correlative imaging spectroscopic methods delivers new insights into the behaviour of materials when treated with ultrashort-pulse laser radiation. Graphical abstract

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A multi-method study of femtosecond laser modification and ablation of amorphous hydrogenated carbon coatings

Hirahara,

Bonse,

Krüger

et al. 2024

Appl. Phys. A

View full text Add to dashboard Cite

show abstract

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Morphology and structure of diamond-like carbon film induced by picosecond laser ablation

Cited by 1 publication

References 20 publications

A multi-method study of femtosecond laser modification and ablation of amorphous hydrogenated carbon coatings

A multi-method study of femtosecond laser modification and ablation of amorphous hydrogenated carbon coatings

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