“…While a photochemical process is usually rapid and precise and can be operated remotely without generating any chemical waste, optofunctional molecules and materials have continueed to attract attention over recent decades. − In particular, chemical systems that are capable of response to visible light are playing an even more significant role in a variety of new appearing fields, − because a visible light source has less harmful effects on the human body as compared with ultraviolet (UV) light and can generally ensure deeper penetration into a large scale of media or biosamples. The past years have witnessed the progress in the visible range of molecular engineering, the application of which has been largely focused on molecular switching, − molecular logic, , molecular assembly, − molecular catalysis, , and so on. − However, the mediation of molecular-scale sensing through visible light has received little attention, probably because the readout of the sensing state of a functional molecule is usually insensitive to visible-light energy; thus, the structural design will meet great challenges.…”