“…[6][7] Especially, owing to their unique physical properties (superconductivity, nonlinear optics, low contact resistance, and intrinsic magnetism), 2D metallic or semimetallic TMDs materials grab considerable attention and show potential applications in 2D electrodes, spintronics, electrocatalysis, and electronic and optoelectronics, etc. [8][9][10][11][12][13][14][15][16] Impressively, 2D metallic or semimetallic-based photodetectors display unique performance in ultrawide band detection, fast response speed, and self-driven operation, owing to the unique energyband structure and Dirac structural characteristics of 2D metal/ semimetals. [17] For instance, the self-powered photodetector based on T d -MoTe 2 shows a broadband photoresponse from 532 nm to 10.6 µm with the responsivity (R) and specific detectivity (D*) of several mA W −1 and 10 6 -10 8 Jones, respectively.…”