Multifunctional macromolecular design as a self-standing electrolyte for high-temperature single-ion lithium batteries

Wang, Yongqin; Zhang, Yanwu; Hou, Hongjun

doi:10.1007/s10800-016-1029-y

J Appl Electrochem

2016

DOI: 10.1007/s10800-016-1029-y

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Multifunctional macromolecular design as a self-standing electrolyte for high-temperature single-ion lithium batteries

Yongqin Wang

Yanwu Zhang

Hongjun Hou

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Cited by 4 publications

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“…The assembled batteries presented superior electrochemical performance. Last, but not least, the ROMP of the norbornene derivative can be employed to construct higher-order structure in SPEs through block, graft, and hyperbranched copolymers. , Thelakkat synthesized a bottlebrush polynorbornene carrying PEG side chains. Compared to linear PEG, the bottlebrush polymer electrolyte exhibits an ionic conductivity 1 order of magnitude higher at 25–80 °C.…”

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confidence: 99%

High Voltage and Cycling Stable Norbornene-Based Polycarbonate Electrolyte for Lithium Metal Battery

Zhang,

Zhao,

Shi

et al. 2024

ACS Materials Lett.

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Solid electrolytes with superb performances, including high ionic conductivity, wide electrochemical window, and optimal compatibility with a lithium (Li) metal anode, would be an efficient solution to the development of nextgeneration high-energy-density Li ion batteries. Herein, a novel polycarbonatebased gel polymer electrolyte (PCPVC-GPE) with high Li + conductivity up to 3.43 mS cm −1 at room temperature is reported. The PCPVC-GPE is synthesized via ringopening metathesis polymerization and thiol−ene "click" chemistry from norbornene derivative monomer exhibiting a high electrochemical oxidation voltage (5.2 V) and superior compatibility with a Li metal anode. A Li/PCPVC-GPE/Li symmetrical cell delivers good cycling stability for 1900 h. As a proof of concept, an assembled Li/PCPVC-GPE/LiFePO 4 cell has a large capacity of 129.4 mAh g −1 at 0.5 C and high capacity retention of 77.1% at 3.0 C after 1000 cycles. All results indicate that PCPVC-GPE could be employed as a promising polymer electrolyte for the advanced solid Li metal batteries.

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mentioning

confidence: 99%

High Voltage and Cycling Stable Norbornene-Based Polycarbonate Electrolyte for Lithium Metal Battery

Zhang,

Zhao,

Shi

et al. 2024

ACS Materials Lett.

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Designing solid-state interfaces on lithium-metal anodes: a review

et al. 2019

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The chemistry of the carbon-transition metal double and triple bond: Annual survey covering the year 2017

Herndon

2018

Coordination Chemistry Reviews

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Multifunctional macromolecular design as a self-standing electrolyte for high-temperature single-ion lithium batteries

Cited by 4 publications

References 37 publications

High Voltage and Cycling Stable Norbornene-Based Polycarbonate Electrolyte for Lithium Metal Battery

High Voltage and Cycling Stable Norbornene-Based Polycarbonate Electrolyte for Lithium Metal Battery

Designing solid-state interfaces on lithium-metal anodes: a review

The chemistry of the carbon-transition metal double and triple bond: Annual survey covering the year 2017

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