Nanoalloy catalysis and magnetic and optical properties: general discussion

Aikens, Christine M.; Amara, Hakim; Amendola, Vincenzo; Baletto, Francesca; Barcikowski, Stephan; Barrabés, Noelia; Caps, Valérie; Chen, Fuyi; Cheng, Daojian; Chinnabathini, Vana Chinnappa; Cottancin, E.; Daniel, Isaac T; Knijf, Kobe De; Fortunelli, Alessandro; Grandjean, D.; Hutchings, Graham J.; Janssens, Ewald; Jones, Robert; Kuttner, Christian; Large, Alex; Marceau, Éric; Mariscal, Marcelo M.; Ntola, Pinkie; Quinson, Jonathan; Shozi, Mzamo; Swaminathan, Swathi; Tréguer‐Delapierre, Mona; Wang, Lichang; Weissker, Hans‐Christian; Yacamán, Miguel José; Zhang, Yufei

doi:10.1039/d2fd90088b

Cited by 1 publication

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“…Through modulation of the structure and composition of the antenna and reactor, their absorption features, catalytic mechanism, and catalytic efficiency of AR systems could be feasibly tuned. [58][59][60][61][62][63][64] In terms of CO 2 reduction, plasmonic AR systems have been found to improve the catalytic performance for different reaction pathways, such as the reverse water gas shift reaction (RWGS), [65][66][67] Sabatier reaction, [68][69][70][71] and dry reforming of methane (DRM). [72][73][74][75] In this review, we systematically overview recent advancements in heterogeneous CO 2 reduction by plasmonic bimetallic AR systems.…”

Section: Introductionmentioning

confidence: 99%

Promises of Plasmonic Antenna‐Reactor Systems in Gas‐Phase CO₂ Photocatalysis

Zhu

Tang

et al. 2023

Advanced Science

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Sunlight‐driven photocatalytic CO2 reduction provides intriguing opportunities for addressing the energy and environmental crises faced by humans. The rational combination of plasmonic antennas and active transition metal‐based catalysts, known as “antenna‐reactor” (AR) nanostructures, allows the simultaneous optimization of optical and catalytic performances of photocatalysts, and thus holds great promise for CO2 photocatalysis. Such design combines the favorable absorption, radiative, and photochemical properties of the plasmonic components with the great catalytic potentials and conductivities of the reactor components. In this review, recent developments of photocatalysts based on plasmonic AR systems for various gas‐phase CO2 reduction reactions with emphasis on the electronic structure of plasmonic and catalytic metals, plasmon‐driven catalytic pathways, and the role of AR complex in photocatalytic processes are summarized. Perspectives in terms of challenges and future research in this area are also highlighted.

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