“…While in some cases the reduction of the dimer exchange may lead to condensation of triplons into sought-for quantum phases of some non-dimerized original model, bilayer systems host their own unique set of physics. For this reason, a variety of bilayer systems have previously been studied under various objectives, e.g., uncovering rich phase diagrams [49][50][51][52][53], examining the crossing to 3D bulk materials [54], investigating effects of disorder [55] and hole doping [56] or analyzing emergent bound states [57] and topological excitations [58]. On the material side, an extensive number of systems exist, which are related to this theme, including Li 2 VOSiO 4 [45], BaCuSi 2 O 6 [59,60], TlCuCl 3 [61], Ba 3 Mn 2 O 8 [62], and SrCu 2 (BO 3 ) 2 [63].…”