Plasmonic modes with long radiative lifetimes combine strong nanoscale light confinement with a narrow spectral line width carrying the signature of Fano resonances, making them very promising for nanophotonic applications such as sensing, lasing, and switching. Their coupling to incident radiation, also known as radiance, determines their optical properties and optimal use in applications. In this work, we theoretically and experimentally demonstrate that the radiance of a plasmonic mode can be classified into three different regimes. In the weak coupling regime, the line shape exhibits remarkable sensitivity to the dielectric environment. We show that geometrical displacements and deformations at the Ångstrom scale can be detected optically by measuring the radiance. In the intermediate regime, the electromagnetic energy stored in the mode is maximal, with large electric field enhancements that can be exploited in surface enhanced spectroscopy applications. In the strong coupling regime, the interaction can result in hybridized modes with tunable energies. KEYWORDS: Fano resonances, electromagnetically induced transparency, plasmonic nanosensors, surface enhanced Raman scattering (SERS), extraordinary optical transmission W ith their ability to concentrate light at a deepsubwavelength scale by excitation of surface plasmons, metallic nanostructures play a major role in current nanoscience. 1 In particular, optical tweezers, 2 antennas, 3,4 lasers, 5 photodetectors, 6 or biochemical sensing platforms 7,8 have been scaled down to the nanometer range. However, their performance are limited by the short lifetimes of surface plasmon resonances. 9 Recently, it has been shown that the use of plasmonic modes with long radiative life times (subradiant modes) can drastically enhance the performance of nanophotonic devices. 10−12 Their spectral response carry an asymmetric line shape with sharp spectral features, characteristic of Fano resonances. 13−22 The coupling of subradiant modes to radiation, their radiance, is directly controlled by the geometrical configuration of the nanostructures, 19 and also governs their optical response and the location and amplitude of light confinement. 20 Despite the fact that the use of subradiant modes for nanophotonic applications critically depends on the coupling strength, the choice of an optimal regime has so far never been addressed.In this work, we use a universal model for interacting radiative and localized channels to investigate the radiance of a plasmonic mode. We demonstrate that the radiance of a plasmonic mode can be classified into three different regimes. In the weak coupling regime, the radiance of the mode is small and extremely sensitive to perturbations in the coupling. We introduce a novel sensing concept, radiance sensing, which is based on the sensitivity of the radiance to the environment, rather than conventional plasmon sensing relying on the wavelength shift of plasmon modes. 8 In the intermediate regime, the radiative damping is equal to the int...