In the past 20 years, impressive progress has been made both experimentally and theoretically in superconducting quantum circuits, which provide a platform for manipulating microwave photons. This emerging field of superconducting quantum microwave circuits has been driven by many new interesting phenomena in microwave photonics and quantum information processing. For instance, the interaction between superconducting quantum circuits and single microwave photons can reach the regimes of strong, ultra-strong, and even deep-strong coupling. Many higher-order effects, unusual and less familiar in traditional cavity quantum electrodynamics with natural atoms, have been experimentally observed, e.g., giant Kerr effects, multi-photon processes, and single-atom induced bistability of microwave photons. These developments may lead to improved understanding of the counterintuitive properties of quantum mechanics, and speed up applications ranging from microwave photonics to superconducting quantum information processing. In this article, we review experimental and theoretical progress in microwave photonics with superconducting quantum circuits. We hope that this global review can provide a useful roadmap for this rapidly developing field.Comment: Review article, 170 pages (main text 101 pages), 35 figures, 5 tables, 1362 references; v2: a few more references added, typos corrected; Physics Reports (in press

Improving the catalytic selectivity of Pd catalysts is of key importance for various industrial processes and remains a challenge so far. Given the unique properties of single-atom catalysts, isolating contiguous Pd atoms into a single-Pd site with another metal to form intermetallic structures is an effective way to endow Pd with high catalytic selectivity and to stabilize the single site with the intermetallic structures. Based on density functional theory modeling, we demonstrate that the (110) surface of Pm3̅m PdIn with single-atom Pd sites shows high selectivity for semihydrogenation of acetylene, whereas the (111) surface of P4/mmm PdIn with Pd trimer sites shows low selectivity. This idea has been further validated by experimental results that intermetallic PdIn nanocrystals mainly exposing the (110) surface exhibit much higher selectivity for acetylene hydrogenation than PdIn nanocrystals mainly exposing the (111) surface (92% vs 21% ethylene selectivity at 90 °C). This work provides insight for rational design of bimetallic metal catalysts with specific catalytic properties.

Some optomechanical systems can be transparent to a probe field when a strong driving field is applied. These systems can provide an optomechanical analogue of electromagnetically-induced transparency (EIT). We study the transmission of a probe field through a hybrid optomechanical system consisting of a cavity and a mechanical resonator with a two-level system (qubit). The qubit might be an intrinsic defect inside the mechanical resonator, a superconducting artificial atom, or another two-level system. The mechanical resonator is coupled to the cavity field via radiation pressure and to the qubit via the Jaynes-Cummings interaction. We find that the dressed twolevel system and mechanical phonon can form two sets of three-level systems. Thus, there are two transparency windows in the discussed system. We interpret this effect as an optomechanical analog of two-color EIT (or double-EIT). We demonstrate how to switch between one and two EIT windows by changing the transition frequency of the qubit. We show that the absorption and dispersion of the system are mainly affected by the qubit-phonon coupling strength and the transition frequency of the qubit.

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