Lasers operating in the blue and yellow-orange spectral regions are sought after by the applications market either to improve well known technologies or to enable new ones. Blue lasers bring features such as high energy photons and smaller diffraction limited beams, while the yellow-orange range is a hard to reach spectral region where there is a considerable shortage of efficient laser light sources. Applications of the blue lasers are found in high density storage technologies, laser displays, LIDAR systems, optical tweezers and a long range of high precision demanding applications. The yellow-orange lasers also have important applications, with highlights in ophthalmologic laser surgery (photocoagulation), in "true" color displays and as a guide star (exciting sodium lines in the atmosphere). The investigation of Nd:YLF quasi-three level lasers and Nd:YLF Raman lasers was further studied in this work in order to provide high power and efficient blue and yellow lasers sources. Demonstrations of efficient and multi-Watt operation of a 908 nm laser and its respective second harmonic laser at 454 nm are described. Also, Nd:YLF/BaWO4 and Nd:YLF/KGW Raman lasers were demonstrated reaching Watt levels in quasi-CW and CW regime with very good beam qualities (M 2 ≤ 2