2020
DOI: 10.1016/j.rinp.2020.103212
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Operation of a bending magnet beamline in large energy bandwidth mode for non-resonant X-ray emission spectroscopy

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Cited by 4 publications
(3 citation statements)
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“…minutes by combining energy-dispersive setups [34] and a high incident X-ray flux. [35] Thus, herein we demonstrate the capability of XES to quantify the average, ex situ spin state of a series of Fe-based M/N/C catalysts (Fe/N/Cs). Furthermore, we show for the first time that XES can track potentialinduced effects on this variable under experimental conditions relevant to the oxygen reduction reaction.…”
mentioning
confidence: 90%
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“…minutes by combining energy-dispersive setups [34] and a high incident X-ray flux. [35] Thus, herein we demonstrate the capability of XES to quantify the average, ex situ spin state of a series of Fe-based M/N/C catalysts (Fe/N/Cs). Furthermore, we show for the first time that XES can track potentialinduced effects on this variable under experimental conditions relevant to the oxygen reduction reaction.…”
mentioning
confidence: 90%
“…This need for techniques that can discriminate oxidation‐ from spin state could potentially be fulfilled by non‐resonant X‐ray emission spectroscopy (XES), [31–33] which additionally allows in situ experiments requiring acquisition over a few minutes by combining energy‐dispersive setups [34] and a high incident X‐ray flux [35] . Thus, herein we demonstrate the capability of XES to quantify the average, ex situ spin state of a series of Fe‐based M/N/C catalysts (Fe/N/Cs).…”
Section: Figurementioning
confidence: 99%
“…Non-resonant XES does not require a monochromatic incident beam, which considerably relaxes the constraints on the X-ray source. At a synchrotron radiation source or freeelectron laser one can use a 'pink' beam with an energy bandwidth much larger than the core-hole lifetime broadening (Dikaya et al, 2020). High-quality Bragg optics have become available at a reasonable cost which has led to the development of instruments by many research groups.…”
Section: Introductionmentioning
confidence: 99%