, many of which can only be realized by confining graphene into nanoribbons and other nanostructures. For example, ballistic room-temperature transistors 3-5 and carbon-based spintronic devices 6-10 are two tantalizing possibilities which could one day be realized in a graphene nanodevice. First though, a reliable method must be found to controllably produce graphene nanostructures with specific sizes, geometries, and defined crystallographic edges. Theoretical predictions indicate that a graphene nanoribbon with zig-zag edges can behave as a half-metal 6, 7 which, paired with graphene's long spin relaxation time 11 , could be used to produced spin-valves and other spintronic devices. In addition, nanosized geometric structures such as triangles with zig-zag edges are predicted to have a net nonzero spin 8,9,12, 13 , furthering the potential use of graphene as a canvas for spintronic circuits. For field effect transistor applications, quantum confinement induces a band gap in the normally gapless graphene 10,14,15 , but the potential performance of the device depends strongly on the edge structure as well 4,16,17 . . Indeed, previous studies of catalytic gasification of carbon found that catalytic metal nanoparticles would sometimes etch graphite along crystallographic directions, creating both armchair and zigzag edges [27][28][29][30][31] .