2012
DOI: 10.1016/s1872-2067(11)60422-1
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Photocatalytic Synthesis of Phenol by Direct Hydroxylation of Benzene by a Modified Nanoporous Silica (LUS-1) under Sunlight

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Cited by 23 publications
(9 citation statements)
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“…To elucidate the effect of sulfur doping and mesoporosity strategies on the photocatalytic activity of the final optimized product, 10 g of urea [undoped g-C 3 N 4 (CN)] and 10 g of thiourea without template [sulfur-doped g-C 3 N 4 without template (CNS)] were separately used for the synthesis of carbon nitrides under the optimized reaction conditions. Moreover, the bulk g-C 3 N 4 sample was synthesized by the condensation of dicyandiamide using the method described in the literature …”
Section: Methodsmentioning
confidence: 99%
See 1 more Smart Citation
“…To elucidate the effect of sulfur doping and mesoporosity strategies on the photocatalytic activity of the final optimized product, 10 g of urea [undoped g-C 3 N 4 (CN)] and 10 g of thiourea without template [sulfur-doped g-C 3 N 4 without template (CNS)] were separately used for the synthesis of carbon nitrides under the optimized reaction conditions. Moreover, the bulk g-C 3 N 4 sample was synthesized by the condensation of dicyandiamide using the method described in the literature …”
Section: Methodsmentioning
confidence: 99%
“…Moreover, the bulk g-C 3 N 4 sample was synthesized by the condensation of dicyandiamide using the method described in the literature. 28 Characterization Techniques. The crystal phases of samples were analyzed by a Philips X'Pert X-ray diffractometer using Cu Kα radiation (k = 1.5406 Å) in the 2θ range of 5−80°.…”
Section: ■ Materials and Methodsmentioning
confidence: 99%
“…In the past several decades, a variety of catalysts have been developed for the direct hydroxylation of benzene with hydrogen peroxide as the oxidant. Various studies have been developed on this reaction using metal-based catalysts on various micro- and mesoporous supports, such as graphitic carbon nitride, activated carbon, and carbon nanotube . Recently, metal-supported mesoporous silica materials were found to be active in the direct oxidation of benzene to phenol because of their high surface area, uniform pore sizes, and large pore volumes. The introduction of transition-metal oxides and their complexes, such as Fe, Cu, and V, into mesoporous supports such as the one-dimensional form of the M41S family has been widely studied.…”
Section: Introductionmentioning
confidence: 99%
“…5,6 Among the various synthetic strategies, hard templating techniques, also known as "nanocasting", using mesoporous silica materials as hard templates are extensively used for the preparation of mesoporous carbon nitride materials. 7,8 Mesoporous carbon nitride materials are widely used in various applications including the aerobic oxidation of alcohols, 9 photocatalytic hydrogen peroxide production, 10 hydrogen and carbon dioxide storage, 11,12 direct hydroxylation of benzene, 13 hydrogen evolution, 14 and CO 2 reduction. 15 However, their application as photoinitiators in free radical polymerization is still at a very early stage, and only a few studies have been reported.…”
Section: Introductionmentioning
confidence: 99%
“…Mesoporous carbon nitride materials are widely used in various applications including the aerobic oxidation of alcohols, photocatalytic hydrogen peroxide production, hydrogen and carbon dioxide storage, , direct hydroxylation of benzene, hydrogen evolution, and CO 2 reduction . However, their application as photoinitiators in free radical polymerization is still at a very early stage, and only a few studies have been reported. , Like other semiconductor materials, combination of the outstanding features of carbon nitride and polymer is expected to positively improve the properties of the obtained composites.…”
Section: Introductionmentioning
confidence: 99%