2009
DOI: 10.1039/b903325d
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Photoelectric conversion switch based on quantum dots with i-motif DNA scaffolds

Abstract: Combining the best features of both inorganic quantum dots and i-motif DNA, a dynamic pH-driven modulation system of photoelectric conversion was realized by making use of their conjugates immobilized on a Au electrode.

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Cited by 45 publications
(30 citation statements)
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“…For example, the distance between the Au electrode and the quantum dots was tuned in situ using the pHsensitive i-motif DNA, resulting in a dynamic pH-driven modulation system for photoelectric conversion. 62 As illustrated in Figure 3a, the Au electrode was modified with an i-motif DNA machine, and the other end of the DNA was connected with CdSe/ZnS core-shell quantum dots. With the switching between acidic and basic conditions, the i-motif machine can change its configuration and bring the quantum dots closer to/further from the Au electrode, respectively, providing a strategy to control dynamically the photoelectric conversion.…”
Section: Dynamic Regulation Of Nps With Dnamentioning
confidence: 99%
“…For example, the distance between the Au electrode and the quantum dots was tuned in situ using the pHsensitive i-motif DNA, resulting in a dynamic pH-driven modulation system for photoelectric conversion. 62 As illustrated in Figure 3a, the Au electrode was modified with an i-motif DNA machine, and the other end of the DNA was connected with CdSe/ZnS core-shell quantum dots. With the switching between acidic and basic conditions, the i-motif machine can change its configuration and bring the quantum dots closer to/further from the Au electrode, respectively, providing a strategy to control dynamically the photoelectric conversion.…”
Section: Dynamic Regulation Of Nps With Dnamentioning
confidence: 99%
“…A photoelectric conversion switch based on quantum dots with i-motif DNA scaffolds is illustrated in Fig. 8 [266]. So far, logic devices, memories, and sensors have all been demonstrated [116,499].…”
Section: Applications Electronicsmentioning
confidence: 99%
“…Photoluminescence colloidal semiconductor nanocrystals, also known as quantum dots, arouse a great interest in fundamental studies and technological applications [1][2][3][4][5][6][7][8][9][10]. As one of the most important II-VI nanocrystals, cadmium selenide (CdSe) becomes a 'model' nanocrystal system for a hotspot of basic studies on the photoelectrical properties of nanocrystals because of its accessibility of high-quality and stability [11].…”
Section: Introductionmentioning
confidence: 99%