2022
DOI: 10.1039/d1cs00859e
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Photoelectrochemical energy storage materials: design principles and functional devices towards direct solar to electrochemical energy storage

Abstract: This review summarizes recent advances in photoelectrochemical energy storage materials and related devices for direct solar to electrochemical energy storage. Design principles, challenges and future developments are specifically highlighted.

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Cited by 166 publications
(120 citation statements)
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References 138 publications
(161 reference statements)
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“…In the photoelectrochemical system, in order to achieve the high performance of the photoelectrode, a large specific surface area is necessary, because it will provide sufficient locations for the photogenerated charge separation in the solar storage device and the load of the dye in SPRBs. [ 60,86 ] Therefore, nanostructured photoelectrodes are usually used. In SPRBs, most photogenerated carriers disappear due to recombination when illuminated.…”
Section: Methods To Improve the Efficiency Of Pecmentioning
confidence: 99%
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“…In the photoelectrochemical system, in order to achieve the high performance of the photoelectrode, a large specific surface area is necessary, because it will provide sufficient locations for the photogenerated charge separation in the solar storage device and the load of the dye in SPRBs. [ 60,86 ] Therefore, nanostructured photoelectrodes are usually used. In SPRBs, most photogenerated carriers disappear due to recombination when illuminated.…”
Section: Methods To Improve the Efficiency Of Pecmentioning
confidence: 99%
“…The poor photoelectric properties of the photoelectrode materials are mainly due to the narrow absorption region of the whole solar spectrum of the materials. [85][86][87] To address this issue which are promising solutions to the dilemma of low photon absorption efficiencies, including narrowing the bandgap and controlling the surface morphology of materials (nanophotonic structures). [39,88,89] For instance, for wide bandgap photoelectrode materials, it is one of the most commonly used methods to enhance the optical absorptivity by doping elements into the photoelectrode to adjust the band structure of the photoelectrode.…”
Section: Enhanced Light Absorptionmentioning
confidence: 99%
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“…[ 3 ] However, these strategies for solar energy usage still face the intrinsic defect of intermittence. [ 4 ] The promising approaches are the simultaneous storage and conversion of solar energy to chemical energy, [ 5 ] including photocatalytic hydrogen production, [ 6 ] CO 2 reduction to solar fuels, [ 7 ] photoelectrochemical conversion of redox couples, [ 8 ] etc. Among them, employing redox couples as the medium to convert and store solar energy is one of the most promising candidates, [ 9 ] because: i) it eliminates the challenges of hydrogen storage and the complicated systems like fuel cells for the subsequent hydrogen utilization; ii) the extremely low CO 2 conversion efficiency and poor products selectivity are not involved; iii) the solar energy conversion and storage as well as the reversible release can be integrated into a single device, making it more flexible and easier for industrial implementation.…”
Section: Introductionmentioning
confidence: 99%
“…It is now crucial to find new, low-cost and environmentally friendly energy conversion and storage systems ( Liu et al, 2020 ). Until now, a great deal of research had been done on energy storage materials and systems ( Duraković and Mešetović, 2019 ; Fleischmann et al, 2020 ; Dou et al, 2021 ; Yang et al, 2021 ; Caturwati et al, 2022 ; Lv et al, 2022 ).…”
Section: Introductionmentioning
confidence: 99%