The optimum preparation conditions for composite snail shell‐rice husk (SS‐RH) adsorbent that gives the optimum brilliant green dye (BGD) uptake has been found at a calcination temperature of 681.10°C, a calcination time of 2.61 hours, and a mixing ratio of 2.61 snail shell‐rice husk, leading to a 97.78% BGD uptake using Central Composite Design. The SS‐RH adsorbent characterization was executed before and after adsorption using a scanning electron microscope (SEM), energy‐dispersive x‐ray spectroscopy (EDS), and Fourier‐transform infrared spectroscopy (FTIR). The SEM image before adsorption showed a highly porous, uniform matrix formation with wide cavities resulting from favorable preparation by calcination at optimum conditions, whereas the image revealed complete adsorption of the BGD onto the vacant pores of the calcined SS‐RH after adsorption. EDS analysis revealed formation of active metal oxides on the surface of the composite SS‐RH was enhanced by the calcination process before adsorption, while changes in their weight percent were noticed after adsorption, showing the influence of the active metal oxides on the process. FTIR revealed the existence of functional groups on the SS‐RH surface, which can interact with the BGD molecules to enhance effective adsorption and cause a shift in the values of the wavenumbers of broad peaks before and after adsorption, respectively. In conclusion, the results obtained have proven SS‐RH to be a valuable composite adsorbent for BGD adsorption.