This paper deals with the study of the enhancement of the tribological properties of AA2024 through the deposition of a titanium coating. In particular two different coatings were studied: (1) untreated titanium coating; and (2) post-deposition laser-treated titanium coating. Titanium grade 2 powders were deposited onto an aluminium alloy AA2024-T3 sheet through the cold gas dynamic spray process. The selective laser post treatment was carried out by using a 220 W diode laser to further enhance the wear properties of the coating. Tribo-tests were executed to analyse the tribological behaviour of materials in contact with an alternative moving counterpart under a controlled normal load. Four different samples were tested to assess the effectiveness of the treatments: untreated aluminium sheets, titanium grade 2 sheets, as-sprayed titanium powders and the laser-treated coating layer. The results obtained proved the effectiveness of the coating in improving the tribological behaviour of the AA2024. In particular the laser-treated coating showed the best results in terms of both the friction coefficient and mass lost. The laser treatment promotes a change of the wear mechanism, switching from a severe adhesive wear, resulting in galling, to an abrasive wear mechanism.