“…The most commonly accepted mechanisms to explain the atmospheric CO 2 decrease include lower sea surface temperatures (Martin et al, 2005;Menviel et al, 2012), iron fertilisation (Bopp et al, 2003;Oka et al, 2011;Jaccard et al, 2013;Ziegler et al, 2013;Martínez-Garcia et al, 2014;Lambert et al, 2015), sea-ice capping of air-sea gas exchange (Stephens and Keeling, 2000;Sun and Matsumoto, 2010;Chikamoto et al, 2012) and ocean circulation/stratification changes (Adkins et al, 2002;20 Lynch-Stieglitz et al, 2007;Skinner et al, 2010;Lippold et al, 2012;Gebbie, 2014;Skinner et al, 2014;Tiedemann et al, 2015;de la Fuente et al, 2015;Freeman et al, 2015), due to a range of possible mechanisms such as increased brine rejection (Shin et al, 2003;Bouttes et al, 2010Bouttes et al, , 2011Zhang et al, 2013;Ballarotta et al, 2014), a shift in/weakening of the westerly wind belt over the Southern Ocean (Toggweiler et al, 2006;Anderson et al, 2009;Völker and Köhler, 2013), stronger westerly winds over the North Atlantic (Muglia and Schmittner, 2015), and a reduced or reversed buoyancy flux from the 25 atmosphere to the ocean surface in the Southern Ocean (Watson and Garabato, 2006;Ferrari et al, 2014). A process that is conversely assumed to have contributed to increasing atmospheric CO 2 is increasing salinity and ocean total dissolved inorganic carbon (DIC) concentration in response to decreasing sea level (Ciais et al, 2013).…”