“…Enhancement of the mid-infrared output power in DFG by use of optical amplifiers, build-up cavities, or laser intracavity DFG typically increases the system cost and complexity, which is disadvantageous in field applications of molecular spectroscopy. Difference-frequency generation in a quasiphase-matched waveguide nonlinear crystal, on the other hand, is an elegant solution to increase the output power without adding much to system cost, size, or complexity [34,42,43,44,45]. A waveguide fabricated in the crystal concentrates the input laser fields in a small mode area of approximately 100 µm 2 .…”