2019
DOI: 10.1029/2019gl084605
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Radiative Forcing and Health Impact of Aerosols and Ozone in China as the Consequence of Clean Air Actions over 2012–2017

Abstract: We applied the chemical transport model GEOS‐Chem to examine the changes in aerosols and tropospheric O3 in China from 2012–2017 and the associated radiative forcing and health impact. Simulated surface layer concentrations and column burdens of aerosols and O3 were evaluated by comparing with ground‐based and satellite‐retrieved measurements. Between 2012 and 2017, simulated annual mean concentrations of PM2.5 decreased by 21.0%, while O3 increased by 11.9% over eastern China (20–45°N, 105–122.5°E). Changes i… Show more

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Cited by 107 publications
(72 citation statements)
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References 57 publications
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“…Most cities in northern, western and southern regions are VOC limited (Sharma et al, 2016), thus this increase in O 3 could be due to more decrease in NOx compared to VOC. Furthermore, this could also be attributed to decrease in PM concentrations, which can result in more sunlight passing through atmosphere encouraging more photochemical activities and thus higher O 3 production (Dang and Liao, 2019;K. Li et al, 2019).…”
Section: Change In Concentrations Of Pollutantsmentioning
confidence: 99%
“…Most cities in northern, western and southern regions are VOC limited (Sharma et al, 2016), thus this increase in O 3 could be due to more decrease in NOx compared to VOC. Furthermore, this could also be attributed to decrease in PM concentrations, which can result in more sunlight passing through atmosphere encouraging more photochemical activities and thus higher O 3 production (Dang and Liao, 2019;K. Li et al, 2019).…”
Section: Change In Concentrations Of Pollutantsmentioning
confidence: 99%
“…3. The contrasting trend of O 3 may be due to more favorable conditions for photochemical reactions attributed to increased solar insolation and a decrease in NO 2 leading to changes in the photochemical reactions determining ozone formation and destruction (Sharma et al, 2016;Dang and Liao, 2019;Xu et al, 2020). The underlying chemistry between anthropogenic emissions like NO x in a VOC-limited environment and O 3 along with the meteorological parameters govern the accumulation of surface ozone in the atmosphere (Gorai et al, 2015;Saini et al, 2017).…”
Section: City Before Vs During Lockdown' 2020mentioning
confidence: 99%
“…The Clean Air Action Plan initiated in 2013 imposed rapid decreases in pollutant emissions (Chinese State Council, 2013) and resulted in large decreases in fine particulate matter (PM 2.5 ) concentrations (Zhai et al, 2019;. However, ozone increased by 1-3 ppb a −1 over the 2013-2017 period in the megacity clusters of eastern China (Lu et al, 2018(Lu et al, , 2020Li et al, 2019a), partly offsetting the health benefits gained from improved PM 2.5 (Dang and Liao, 2019;. Phase 2 of the Clean Air Action Plan, which began in 2018 (Chinese State Council, 2018), imposed new emission controls targeted at ozone.…”
Section: Introductionmentioning
confidence: 99%