2021
DOI: 10.1021/acsami.0c17525
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Rapid Moisture-Responsive Silk Fibroin Actuators

Abstract: We report the unique actuation characteristics of moisture-driven, fully reversible soft biopolymer films fabricated from Bombyx mori silk. The instantaneous actuation is driven by the water vapor induced stress gradient generated across the thickness of the film, and it possesses subsecond response and actuation times. The excellent durability and consistent performance of the film without any noticeable fatigue are established by subjecting it to more than a thousand continuous actuation cycles. The weight-l… Show more

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Cited by 47 publications
(53 citation statements)
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“…[ 23 , 24 ] Meanwhile, CNT has a small CTE (16–26 ppm K −1 ). [ 25 , 26 ] And the silk expands by absorbing water, [ 20 , 27 ] thus it loses water and shrinks when heated. When the CNT–Silk/BOPP actuator is driven by a voltage, the highly conductive CNT–Silk layer is used as an electrothermal heating component.…”
Section: Resultsmentioning
confidence: 99%
“…[ 23 , 24 ] Meanwhile, CNT has a small CTE (16–26 ppm K −1 ). [ 25 , 26 ] And the silk expands by absorbing water, [ 20 , 27 ] thus it loses water and shrinks when heated. When the CNT–Silk/BOPP actuator is driven by a voltage, the highly conductive CNT–Silk layer is used as an electrothermal heating component.…”
Section: Resultsmentioning
confidence: 99%
“…For this reason, PDMS and other silicone‐based electronic applications also may contain silk fibroin. [ 242 ] In addition to silkworm sourced ones, silk fibroin produced by the spider species with carbon nanotube coating was reported in sensing and actuating applications. [ 243 ]…”
Section: Sustainable Materials In Flexible Electronicsmentioning
confidence: 99%
“…This excellent actuation property enables the spider web to maintain its geometric configuration in a changing environment and even allows the spider to perceive the external load imposed on the web. [ 25 ] B. mori silk fibers have a molecular structure similar to that of spider silk proteins [ 125 ] and the ability to lift a small load through humidity‐induced cyclic contraction and expansion. Therefore, many studies have been conducted on humidity‐triggered silk fiber (yarn) actuators.…”
Section: Meso‐functionalized Silk Fibrous Devices and Applicationsmentioning
confidence: 99%