2021
DOI: 10.1002/inf2.12257
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Rational confinement engineering of MOF‐derived carbon‐based electrocatalysts toward CO2 reduction and O2 reduction reactions

Abstract: The goal of global carbon peak and neutrality gives an impetus to the utilization of clean energy (e.g., fuel cell) and carbon dioxide (CO 2 ) at a large scale, where the oxygen reduction reaction (ORR) and CO 2 reduction reaction (CO 2 RR) are the key reactions via the sustainable system, respectively. As a main precursor for fabricating affordable carbon-based electrocatalysts with uniformly dispersed active centers and tailorable performances for ORR and CO 2 RR, metal organic frameworks (MOFs) have capture… Show more

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Cited by 81 publications
(34 citation statements)
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“…The size of the fabricated material was determined with Debye Scherrer eq. 7. [51–56] D=boldKλβboldcboldoboldsθ $\vcenter{\openup.5em\halign{$\displaystyle{#}$\cr {\bf D}={\rm \ }{{{\bf K \lambda }{\rm \ }}\over{{\bf \beta c o s}{\rm \ }{\bf \theta }{\rm \ }}}\hfill\cr}}$ …”
Section: Resultsmentioning
confidence: 99%
“…The size of the fabricated material was determined with Debye Scherrer eq. 7. [51–56] D=boldKλβboldcboldoboldsθ $\vcenter{\openup.5em\halign{$\displaystyle{#}$\cr {\bf D}={\rm \ }{{{\bf K \lambda }{\rm \ }}\over{{\bf \beta c o s}{\rm \ }{\bf \theta }{\rm \ }}}\hfill\cr}}$ …”
Section: Resultsmentioning
confidence: 99%
“…Another critical parameter in ORR electrocatalysts is long-term stability. A stable electrocatalyst means that the catalyst can maintain its activity for a period of time . The ORR stability can be measured by applying a constant potential or current (i.e., chronoamperometry or chronopotentiometry).…”
Section: Mechanism Of Orr In Different Ph Electrolytesmentioning
confidence: 99%
“…A stable electrocatalyst means that the catalyst can maintain its activity for a period of time. 119 The ORR stability can be measured by applying a constant potential or current (i.e., chronoamperometry or chronopotentiometry). Afterward, a change in the output response (current or voltage) as a function of time is recorded, where stable electrocatalysts would yield a low output loss rate.…”
Section: Parameters Of Orr Activity and Stabilitymentioning
confidence: 99%
“…24,25 Meanwhile, porous carbon-based materials with unique characteristics are also considered favourable catalysts or support for electrocatalysis. 26 Metal-organic frameworks (MOFs) have been studied a lot in recent years due to the large surface area and tuneable structure by variation of the metal cation and organic linkers. [27][28][29] However, the instability of MOFs restricts their catalytic performance.…”
Section: Introductionmentioning
confidence: 99%