With the active development of offshore wind power worldwide, the development of a green and ecofriendly grouting material (GEGM) has garnered global attention. Such a material must also be developed in Taiwan. Therefore, in this study, a series of environmentally friendly recycled materials were mixed in different proportions to develop a GEGM which can be implemented in the future construction of offshore wind turbines. To evaluate the mechanical properties of the GEGM, low water-to-binder (W/B) ratios (i.e., 0.21, 0.27, and 0.35) were used; cement was replaced with fixed amounts (20%) of ground granulated blast-furnace slag and fly ash; 2%, 2.5%, and 3% superplasticizers (SPs) were added; and two levels of sand content (60% and 70%) were used. The setting time of the GEGM was used to evaluate its workability; its compressive strength and flexural strength were used to evaluate its mechanical properties; and its sulfate resistance, length changes, and four-terminal resistance were used to evaluate its durability. The relationship between the durability and drying shrinkage of the GEGM was subsequently evaluated, and the ratio of final to initial setting times (F/I value) was calculated to determine the effects of the amount of SP added on workability. The highest F/I value (7.7) was achieved when 2 wt.% modified lignin sulfonate (MLS) was added because of the high viscosity of MLS, which compromised the workability of the concrete. The optimal compressive strength (83.62 MPa) was achieved when a W/B ratio of 0.21 was used, when the sand content was 70%, and when a 2% polycarboxylate superplasticizer (PCE) was added, whereas the optimal flexural strength (20.86 MPa) was achieved when 2.5% PCE was added. According to the nondestructive test results and the R2 value (>0.7) obtained from regression analyses of mechanical properties, the study results are reliable and may serve as a reference for future construction projects.