3D metamaterials, has attracted considerable attention given its unique optical properties and produced many new phenomena and functionalities, such as plate focusing, [8] polarization conversion, [9] and mathematical operations. [10,11] The construction of these optical metasurfaces is generally a periodic arrangement of metal or dielectric micro-nanostructures. On the basis of the requirements, a plurality of the structural units with different geometric parameters (such as shape, size, and orientation) is arranged in an array to realize various kinds of abnormal optical responses. [12] However, few experimental reports are presented on periodic metasurfaces that respond in visible light. Cost remains high, large-area preparation remains challenging, and the deviation of the prepared structure is large, although tens of nanometer-sized structures can be prepared using complex electron beam-or ion beam-etching techniques, [13,14] thereby making periodic metasurfaces difficult to be extensively applied. The design requirement of periodic structures for the existing metasurfaces and top-down electron beam or ion beam etching technology, as well as the unidirectionality of optical response for the periodic metasurfaces, have become the bottlenecks that limit the rapid development of optical metasurfaces.Recently, researchers have used the Gerchberg-Saxton (GS) algorithm [15] to iterate a random-phase profile and obtain a disordered metasurface with a convergent-phase profile that manipulates the transmission of visible light and allows a farfield pattern to have isotropic scattering over a desired angular range. [16] To a certain extent, this method simplifies the preparation of optical metasurfaces. However, its structure must be prepared by electron beam lithography. Thus, this method does not completely solve the constraint that restrains the development of optical metasurfaces.Inspired by the idea of the GS algorithm, [15] we propose a quasiperiodic dendritic cluster set metasurface. In the simulation, the periodic metasurface tends toward the quasiperiodic metasurface by gradually changing the state of the dendritic structure in the periodic structural unit; in the bottom-up electrochemical deposition experiment, the disordered distribution of dendritic cluster sets tends toward the quasiperiodic distribution by continuously adjusting the preparation conditions. By gradually changing the theoretical model from a periodic structure to a quasiperiodic structure and the distribution of dendritic cluster sets in the sample from a disordered distribution Periodic metasurfaces have achieved various light manipulations. However, the preparation of those responding in visible waveband still encounters many constraints. Inspired by the idea of the Gerchberg-Saxton algorithm, a quasiperiodic dendritic cluster set metasurface is proposed where the cluster is used as the unit instead of cell that is used as the unit in the periodic metasurface. By gradually changing the theoretical model from periodic to quasiperiodic str...